Facile Synthesis of Organically Synthesized Porous Carbon Using a Commercially Available Route with Exceptional Electrochemical Performance.

Organically synthesized porous carbon (OSPC) is a subclass of conjugated microporous polymer materials that have shown potential applications as anodes in ion batteries. However, a challenging, low-yielding, multistep synthetic route (the A method) has hindered further exploration of this exciting family. Here, OSPC-1 has been synthesized via an alternative, efficient one-pot method from commercially available reagents (the B method), hereafter referred to as OSPC-1b in contrast to OSPC-1a, where it is synthesized via the A method.

Artificial synthesis of covalent triazine frameworks for local structure and property determination.

Here we show an 'artificial synthesis' method for covalent triazine framework (CTF) materials, enabling localised structural features to be incorporated that result directly from the acid-catalysed synthetic protocol that would otherwise not be captured. This advancement will enable prediction and design of new CTF materials with targeted properties.