We report an experimental and theoretical study of light emission by a patterned ensemble of colloidal quantum dots (cQDs). This system modifies drastically the emission spectrum and polarization as compared to a planar layer of cQDs. It exhibits bright, directional and polarized emission including a degree of circular polarization in some directions.
View Article and Find Full Text PDFIn semiconductor nanocrystals, excited electrons relax through multiple radiative and nonradiative pathways. This complexity complicates characterization of their decay processes with standard time- and temperature-dependent photoluminescence studies. Here, we exploit a simple nanophotonic approach to augment such measurements and to address open questions related to nanocrystal emission.
View Article and Find Full Text PDFColloidal quantum-dots (cQDs) are finding increasingly widespread application in photonics and optoelectronics, providing high brightness and record-wide colour gamuts. However, the external quantum efficiencies in thin-film device architectures are still limited due to losses into waveguide modes and different strategies are being explored to promote the outcoupling of emission. Here we use a template-stripping-based direct-patterning strategy to fabricate linear gratings at the surface of cQD thin films.
View Article and Find Full Text PDFThe pursuit of miniaturized optical sources for on-chip applications has led to the development of surface plasmon polariton lasers (plasmonic lasers). While applications in spectroscopy and information technology would greatly benefit from the facile and active tuning of the output wavelength from such devices, this topic remains underexplored. Here, we demonstrate optically controlled switching between predefined wavelengths within a plasmonic microlaser.
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