Studying the dynamics of dark states is challenging due to their inability to undergo single-photon emission or absorption. This challenge is made even more difficult for dark autoionizing states owing to their ultrashort lifetime of a few femtoseconds. High-order harmonic spectroscopy recently appeared as a novel method to probe the ultrafast dynamics of a single atomic or molecular state.
View Article and Find Full Text PDFAn approach for accelerating ions, with the use of a cluster-gas target and an ultrashort pulse laser of 150-mJ energy and 40-fs duration, is presented. Ions with energy 10-20 MeV per nucleon having a small divergence (full angle) of 3.4 degrees are generated in the forward direction, corresponding to approximately tenfold increase in the ion energies compared to previous experiments using solid targets.
View Article and Find Full Text PDFPhys Rev E Stat Nonlin Soft Matter Phys
June 2006
A model that solves simultaneously both the electron and atomic kinetics was used to generate a synthetic He alpha and satellite x-ray spectra to characterize a high intensity ultrashort laser driven Ar cluster target experiment. In particular, level populations were obtained from a detailed collisional-radiative model where collisional rates were computed from a time varying electron distribution function obtained from the solution of the zero-dimensional Boltzmann equation. In addition, a particle-in-cell simulation was used to model the laser interaction with the cluster target and provided the initial electron energy distribution function (EEDF) for the Boltzmann solver.
View Article and Find Full Text PDFPhys Rev E Stat Nonlin Soft Matter Phys
June 2006
We diagnose the self-channeled propagation of intense femtosecond pulses over an extended distance in a N2O cluster gas target using high resolution kilovolt x-ray pinhole images of the channel and spatially resolved x-ray spectra. The x-ray images are consistent with femtosecond optical scattering, shadowgraphy, and interferometry images. We observe extended plasma channels (approximately 9 mm) limited either by the cluster jet length or by absorption, for injected laser intensities in the range of 10(16)-10(17) W/cm2.
View Article and Find Full Text PDFPhys Rev E Stat Nonlin Soft Matter Phys
January 2005
X-ray line emission from 2l-nl' transitions in Ne-like Kr and nearby ions has been observed from approximately 1 microm Kr clusters irradiated by fs-scale laser pulses at the JAERI facility in Kyoto, Japan. The incident laser intensity reached 10(19) W/cm2, with pulse energies from 50 to 300 mJ and pulse durations from 30 to 500 fs. The dependence of the x-ray spectral features and intensity on the incident laser intensity is rather weak, indicating that the 1-2 ps cluster lifetimes limit the number of ions beyond Ne-like Kr that can be produced by collisional ionization.
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